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Walter Kmak Phones & Addresses

  • Potomac, MD
  • Gaithersburg, MD
  • Scotch Plains, NJ
  • Alexandria, VA

Publications

Us Patents

Process For Reactivating An Iridium-Containing Catalyst

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US Patent:
41728173, Oct 30, 1979
Filed:
May 22, 1978
Appl. No.:
5/907928
Inventors:
David J. C. Yates - Bernards Township, Somerset County NJ
Walter S. Kmak - Scotch Plains NJ
Assignee:
Exxon Research & Engineering Co. - Florham Park NJ
International Classification:
C10G 3508
US Classification:
208140
Abstract:
This invention relates to improvements in a process for treating a catalyst, or bed of catalyst, comprised of a composite of an iridium metal or admixture of said metal with other metals, particularly platinum, or admixtures of iridium and platinum with other metals, halogen, and a refractory porous inorganic oxide, notably alumina which has been deactivated by coke deposition thereon, as commonly occurs in a hydroconversion reactions, notably as in upgrading virgin or cracked naphthas in catalytic reforming to produce higher octane products. The time required for reactivation of such catalyst can be shortened by deliberate agglomeration of the iridium, or admixture of iridium and other metal hydrogenation-dehydrogenation components, above about seventy percent, and preferably by essentially complete agglomeration of the iridium, or admixture of iridium and other metal hydrogenation-dehydrogenation components, prior to one or more cycles of sequential reduction/halogenation treatments. The desired high agglomeration of the iridium, or admixture of iridium and other metal hydrogenation-dehydrogenation components, is preferably accomplished by a relatively severe coke burn which not only achieves the desired agglomeration, but also more efficiently and effectively removes the coke from the coked catalyst.

Method Of Minimizing Iron Contamination During Catalyst Regeneration Processes

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US Patent:
60340193, Mar 7, 2000
Filed:
Sep 8, 1997
Appl. No.:
8/925519
Inventors:
Shun C. Fung - Bridgewater NJ
Walter S. Kmak - Scotch Plains NJ
Assignee:
Exxon Research and Engineering Co. - Florham Park NJ
International Classification:
B01J 2034
US Classification:
502 35
Abstract:
The present invention is directed toward improved processes for the regeneration of noble metal-containing catalysts wherein iron contamination of the catalyst during regeneration is significantly diminished. It has been found that maintenance of any iron present in contact with the catalyst in the oxidized state (e. g. , as Fe. sub. 2 O. sub. 3 or Fe. sub. 3 O. sub. 4) during contact of the catalyst with a source of halogen in the regeneration haliding step results in a marked decrease in the degree of catalyst contamination by iron species.

Regeneration Procedure

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US Patent:
39430529, Mar 9, 1976
Filed:
Aug 16, 1973
Appl. No.:
5/388743
Inventors:
Walter S. Kmak - Scotch Plains NJ
David J. C. Yates - Westfield NJ
Assignee:
Exxon Research & Engineering Co. - Linden NJ
International Classification:
C10G 3508
B01J 2396
US Classification:
208140
Abstract:
Supported iridium-containing hydrocarbon conversion catalysts which are at least partially deactivated due to the deposition of carbonaceous residues thereon during contact with hydrocarbons are regenerated by (1) contacting the catalyst with oxygen to burn at least a portion of the carbonaceous residues from the catalyst, (2) contacting the carbonaceous residue-depleted catalyst with an elemental halogen-containing gas at a temperature of less than about 850. degree. F. , (3) contacting the treated catalyst with hydrogen at elevated temperatures to reduce a substantial portion of the iridium present in the catalyst to its metallic form, and (4) contacting the catalyst from step (3) with an elemental halogen-containing gas at a temperature of at least about 850. degree. F. Steps (3) and (4) may be repeated, in sequence, at least one additional time to redisperse the iridium catalyst component to a highly active, high surface area state.

Method Of Minimizing Iron Contamination During Catalyst Regeneration Processes

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US Patent:
6110857, Aug 29, 2000
Filed:
Sep 8, 1997
Appl. No.:
8/925364
Inventors:
Shun C. Fung - Bridgewater NJ
Walter S. Kmak - Scotch Plains NJ
Assignee:
Exxon Research and Engineering Company - Florham Park NJ
International Classification:
B01J 2034
US Classification:
502 35
Abstract:
The present invention is directed toward improved processes for the regeneration of noble metal-containing catalysts wherein iron contamination of the catalyst during regeneration is significantly diminished. It has been found that maintenance of any iron present in contact with the catalyst in the oxidized state (e. g. , as Fe. sub. 2 O. sub. 3 or Fe. sub. 3 O. sub. 4) during contact of the catalyst with a source of halogen in the regeneration haliding step results in a marked decrease in the degree of catalyst contamination by iron species.

Method For Removing Coronene From Heat Exchangers

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US Patent:
42038251, May 20, 1980
Filed:
Feb 2, 1979
Appl. No.:
6/008777
Inventors:
Walter S. Kmak - Scotch Plains NJ
Charles Monzo - Sea Brook TX
Assignee:
Exxon Research & Engineering Co. - Florham Park NJ
International Classification:
C07C 1512
C10G 916
C10G 3900
US Classification:
208 48R
Abstract:
Coronene deposits are removed from a heat exchange zone of a reforming process by operating the reforming zone at conditions such that at least a portion of the reformer effluent condenses in the heat exchange zone where the coronene deposit occurs.

Method For Removing Coronene From Heat Exchangers

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US Patent:
42149762, Jul 29, 1980
Filed:
Feb 2, 1979
Appl. No.:
6/009228
Inventors:
Walter S. Kmak - Scotch Plains NJ
Assignee:
Exxon Research & Engineering Co. - Florham Park NJ
International Classification:
C10G 916
C10G 3900
C07C 1512
US Classification:
208 48R
Abstract:
Coronene deposits are removed from a heat exchange zone disposed in two parallel trains of heat exchangers in a reforming process by reducing the flow of reforming zone effluent in one of the trains of heat exchangers sufficiently to effect condensation of a portion of the reforming zone effluent in said one train of heat exchangers where the coronene is deposited while simultaneously increasing the flow of reforming zone effluent in the second train of heat exchangers. Control means are provided in each of the heat exchange trains.

Method For Removing Coronene From Heat Exchangers

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US Patent:
42228522, Sep 16, 1980
Filed:
Feb 2, 1979
Appl. No.:
6/009229
Inventors:
Walter S. Kmak - Scotch Plains NJ
Akira Yatabe - Lake Hiawatha NJ
Assignee:
Exxon Research & Engineering Co. - Florham Park NJ
International Classification:
C10G 916
C10G 3900
C07C 1512
US Classification:
208 48R
Abstract:
Coronene deposits are removed from a heat exchange zone of the reforming process by recycling a portion of the normally liquid reformate to the heat exchange zone to dissolve the coronene deposits.

Reactivating Iridium-Containing Catalysts With Hydrogen Halide And Oxygen

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US Patent:
44448970, Apr 24, 1984
Filed:
May 5, 1982
Appl. No.:
6/374978
Inventors:
Shun C. Fung - Bridgewater NJ
Walter Weissman - Berkeley Heights NJ
James L. Carter - Westfield NJ
Walter S. Kmak - Scotch Plains NJ
Assignee:
Exxon Research and Engineering Co. - Florham Park NJ
International Classification:
B01J 2396
B01J 2346
B01J 2364
C10G 35085
US Classification:
502 37
Abstract:
A process is disclosed for reactivating an agglomerated iridium-containing catalyst and particularly platinum-iridium on alumina reforming catalysts. The process includes contacting a substantially decoked agglomerated catalyst with a reducing gas such as hydrogen to reduce agglomerated iridium oxides present to the free metal, a hydrogen halide pretreatment step to increase the halogen level of the catalyst to about 1. 3 weight percent and above, and a redispersion step involving hydrogen halide and elemental oxygen. Use of hydrogen halide and elemental oxygen in the redispersion treatment eliminates the need for use of elemental chlorine gas. If no iridium oxides are initially present, the hydrogen reduction step is optional.
Walter S Kmak from Potomac, MDDeceased Get Report